For PC players, there is a sneaky workaround to make this achievement muuuch easier, one very similar to the workaround for the LASO and Par Time/Score achievements. For each level, do the following:
*Enable whatever mods or cheats you want by launching the game with Anti-Cheat enabled (or "mod mode," as I call it). You can't earn achievements in mod mode, but it will still save your mission checkpoints.
*Start the given level on Legendary (I also had some skulls on because I was going for the par score achievements as well). Be sure to turn scoring or time on.
*Run through the level as quickly as you can only killing what you really need to.
**The mod I was using gave me infinite shields, ammo, and let me kill most enemies instantaneously, so it was not difficult in the slightest. I won't link to the mod here, so all I'll say is that google is your friend.
*During the ending cutscene, press
to bring up the menu (this will pause the cutscene, you don't want to skip it), and select Save/Quit.
*Close the game and relaunch it with anti-cheat enabled (which will let you earn achievements).
*Once the level loads, you should be taken to the postgame carnage report (which is why you need time enabled), and the game will upload your time to your service record (which you can check on https://www.halowaypoint.com/en-us
Do this for all nine main levels (Noble Actual and Epilogue don't count). Then play Lone Wolf on Legendary without mods, off yourself as quickly as you can, and the achievement is yours. If you take some extra time to kill extra enemies, you can easily get the Par Score achievements as well. It really is as simple as that.
This is very much an exploit with the way "mod mode" works on the PC version, but given that you still have to play through the levels on the highest difficulty and do them quickly, it is still well within the site's rules (and Microsoft's ToS). Mind you, a similar solution regarding the LASO achievement was vetted by the site mods. If you want to do these the traditional way, go for it, this is primarily for those of us who don't have the time or patience for grinding these out one at a time.